Since it
IS a
moving iron meter, instead of a moving coil, removing turns of wire from the coil should not increase the "sensitivity" but instead decrease the inductance of the coil, as well as decreasing the magnetic field produced when current flows through the coil, and hence the reactive force of the iron vane (attached to the needle) that responds to coil current.
It is highly doubtful that the original installation passed anything near 500 A through this meter. It was probably connected to a calibrated shunt whose voltage drop was then applied as excitation to the meter. Or it may have been connected to a current transformer. In either case, the non-linearity at either end of the scale is indicative of a meter designed to measure AC. The iron vane may not respond to higher audio frequencies, but it should be okay for the lower bass frequencies up to 100 Hz or so.
So, go ahead and "experiment" with your 9 V battery and find out how much voltage and current you need to deflect the needle as far as you want for the effect you are seeking. Then buy or build an audio amplifier capable of producing that much voltage and current. If that is a problem (getting sufficient voltage) you can connect a 6.3 VAC filament transformer "backwards" to the amplifier output, driving the 6.3 VAC secondary winding with the audio amplifier and driving the meter from the primary winding. The meter won't require much current, so the smallest filament transformer you can buy or salvage should be fine.
This should make a nice steam punk "hi-fi" installation. I am envious.